Um...I can only really think of two off the top of my head. Kagura from 'Fruits Basket' and Dokora-chan from 'Bokusatsu Tenshi Dokuro-chan' - she's not so much psychotic, just over powered...but on the other hand, anyone who can kill someone without a second thought (even if they can bring them back to life afterwards) definitely falls under the 'unhinged' category.
Kagura is probably the best example of a yandere, but I'm not sure she's my favourite. I think the winner is Akane from 'Kampfer'...
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